Ok, I think people should really distinguish between KB and Kb. The first is mostly used to say KByte and the later to say Kbit. As far as I can see, there are only TWO chips used as a VRAM for the VDC chipset. So we are speaking about turning 2 x 16K x 4 bits into 2 x 64K x 4 bits. Let see the pin layout of those chips:
PIN 16K x 4bit (4416?) 64K x 4bit (41464)
1 nOE nOE
2 DATA DATA
3 DATA DATA
4 nWE nWE
5 nRAS nRAS
6 ADDR ADDR
7 ADDR ADDR
8 ADDR ADDR
9 VCC VCC
10 ADDR ADDR
11 ADDR ADDR
12 ADDR ADDR
13 ADDR ADDR
14 ADDR ADDR
15 DATA DATA
16 nCAS nCAS
17 DATA DATA
18 GND GND
Their pins match (data and address order don't matter).
I suppose if you try to access beyond 16KB with a 16KB version, you may have a mirrored 16KB or random bytes.
Well, I guess it is safe to swap them indeed.
As for the solder-less plug-in, I'm not expecting it to be safe because I wonder how the plugin is shutting the original RAM chips and how it tries to reroute some data. As for the capacity on the plugin board, it may be needed between a pin of the VDC chip and a pin of the two new RAM chips.